Zhu Liu

Tao Li, Lixing Wang, Zihan Qiu et al.

High temporal resolution CO2 emission data are crucial for understanding the drivers of emission changes, however, current emission dataset is only available on a yearly basis. Here, we extended a global daily CO2 emissions dataset backwards in time to 1970 using machine learning algorithm, which was trained to predict historical daily emissions on national scales based on relationships between daily emission variations and predictors established for the period since 2019. Variation in daily CO2 emissions far exceeded the smoothed seasonal variations. For example, the range of daily CO2 emissions equivalent to 31% of the year average daily emissions in China and 46% of that in India in 2022, respectively. We identified the critical emission-climate temperature (Tc) is 16.5 degree celsius for global average (18.7 degree celsius for China, 14.9 degree celsius for U.S., and 18.4 degree celsius for Japan), in which negative correlation observed between daily CO2 emission and ambient temperature below Tc and a positive correlation above it, demonstrating increased emissions associated with higher ambient temperature. The long-term time series spanning over fifty years of global daily CO2 emissions reveals an increasing trend in emissions due to extreme temperature events, driven by the rising frequency of these occurrences. This work suggests that, due to climate change, greater efforts may be needed to reduce CO2 emissions.

Zhu Deng, Jinjie Liu, Biao Luo et al.

The product carbon footprint (PCF) is crucial for decarbonizing the supply chain, as it measures the direct and indirect greenhouse gas emissions caused by all activities during the product's life cycle. However, PCF accounting often requires expert knowledge and significant time to construct life cycle models. In this study, we test and compare the emergent ability of five large language models (LLMs) in modeling the 'cradle-to-gate' life cycles of products and generating the inventory data of inputs and outputs, revealing their limitations as a generalized PCF knowledge database. By utilizing LLMs, we propose an automatic AI-driven PCF accounting framework, called AutoPCF, which also applies deep learning algorithms to automatically match calculation parameters, and ultimately calculate the PCF. The results of estimating the carbon footprint for three case products using the AutoPCF framework demonstrate its potential in achieving automatic modeling and estimation of PCF with a large reduction in modeling time from days to minutes.

Risheng Liu, Zhu Liu, Wei Yao et al.

This work focuses on addressing two major challenges in the context of large-scale nonconvex Bi-Level Optimization (BLO) problems, which are increasingly applied in machine learning due to their ability to model nested structures. These challenges involve ensuring computational efficiency and providing theoretical guarantees. While recent advances in scalable BLO algorithms have primarily relied on lower-level convexity simplification, our work specifically tackles large-scale BLO problems involving nonconvexity in both the upper and lower levels. We simultaneously address computational and theoretical challenges by introducing an innovative single-loop gradient-based algorithm, utilizing the Moreau envelope-based reformulation, and providing non-asymptotic convergence analysis for general nonconvex BLO problems. Notably, our algorithm relies solely on first-order gradient information, enhancing its practicality and efficiency, especially for large-scale BLO learning tasks. We validate our approach's effectiveness through experiments on various synthetic problems, two typical hyper-parameter learning tasks, and a real-world neural architecture search application, collectively demonstrating its superior performance.

Xinyu Dou, Cuijuan Liao, Hengqi Wang et al.

Nitrogen dioxide (NO2) is one of the most important atmospheric pollutants. However, current ground-level NO2 concentration data are lack of either high-resolution coverage or full coverage national wide, due to the poor quality of source data and the computing power of the models. To our knowledge, this study is the first to estimate the ground-level NO2 concentration in China with national coverage as well as relatively high spatiotemporal resolution (0.25 degree; daily intervals) over the newest past 6 years (2013-2018). We advanced a Random Forest model integrated K-means (RF-K) for the estimates with multi-source parameters. Besides meteorological parameters, satellite retrievals parameters, we also, for the first time, introduce socio-economic parameters to assess the impact by human activities. The results show that: (1) the RF-K model we developed shows better prediction performance than other models, with cross-validation R2 = 0.64 (MAPE = 34.78%). (2) The annual average concentration of NO2 in China showed a weak increasing trend . While in the economic zones such as Beijing-Tianjin-Hebei region, Yangtze River Delta, and Pearl River Delta, the NO2 concentration there even decreased or remained unchanged, especially in spring. Our dataset has verified that pollutant controlling targets have been achieved in these areas. With mapping daily nationwide ground-level NO2 concentrations, this study provides timely data with high quality for air quality management for China. We provide a universal model framework to quickly generate a timely national atmospheric pollutants concentration map with a high spatial-temporal resolution, based on improved machine learning methods.