Shen Zhou

Wenqiang Huang, Susu Fang, Xuhang Gu et al.

Exemplified by the chemical vapor deposition growth of two-dimensional dendrites, which has potential applications in catalysis and presents a parameter-intensive, data-scarce and reaction process-complex model problem, we devise a machine intelligence-empowered framework for the full chain support of material synthesis, encompassing rapid process optimization, accurate customized synthesis, and comprehensive mechanism deciphering.First, active learning is integrated into the experimental workflow, identifying an optimal recipe for the growth of highly-branched, electrocatalytically-active ReSe2 dendrites through 60 experiments (4 iterations), which account for less than 1.3% of the numerous possible parameter combinations.Then, a prediction accuracy-guided data augmentation strategy is developed combined with a tree-based machine learning (ML) algorithm, unveiling a non-linear correlation between 5 process variables and fractal dimension (DF) of ReSe2 dendrites with only 9 experiment additions, which guides the synthesis of various user-defined DF. Finally, we construct a data-knowledge dual-driven mechanism model by integration of cross-scale characterizations, interpretable ML models, and domain knowledge in thermodynamics and kinetics, unraveling synergistic contributions of multiple process parameters to the product morphology. This work demonstrates the ML potential to transform the research paradigm and is adaptable to broader material synthesis.

Mayi Xu, Yunfeng Ning, Yongqi Li et al.

Reasoning is fundamental to human intelligence, and critical for problem-solving, decision-making, and critical thinking. Reasoning refers to drawing new conclusions based on existing knowledge, which can support various applications like clinical diagnosis, basic education, and financial analysis. Though a good number of surveys have been proposed for reviewing reasoning-related methods, none of them has systematically investigated these methods from the viewpoint of their dependent knowledge base. Both the scenarios to which the knowledge bases are applied and their storage formats are significantly different. Hence, investigating reasoning methods from the knowledge base perspective helps us better understand the challenges and future directions. To fill this gap, this paper first classifies the knowledge base into symbolic and parametric ones. The former explicitly stores information in human-readable symbols, and the latter implicitly encodes knowledge within parameters. Then, we provide a comprehensive overview of reasoning methods using symbolic knowledge bases, parametric knowledge bases, and both of them. Finally, we identify the future direction toward enhancing reasoning capabilities to bridge the gap between human and machine intelligence.