Deep learning-based denoising for fast time-resolved flame emission spectroscopy in high-pressure combustion environment
This work addresses the challenge of accurate gas property measurements in combustion research, though it appears incremental as it builds on existing denoising CNNs with specific architectural and loss function modifications.
The paper tackles the problem of low signal-to-noise ratio in fast time-resolved flame emission spectroscopy for high-pressure combustion, proposing a deep learning-based denoising method that reduces property prediction errors for pressure and equivalence ratio.
A deep learning strategy is developed for fast and accurate gas property measurements using flame emission spectroscopy (FES). Particularly, the short-gated fast FES is essential to resolve fast-evolving combustion behaviors. However, as the exposure time for capturing the flame emission spectrum gets shorter, the signal-to-noise ratio (SNR) decreases, and characteristic spectral features indicating the gas properties become relatively weaker. Then, the property estimation based on the short-gated spectrum is difficult and inaccurate. Denoising convolutional neural networks (CNN) can enhance the SNR of the short-gated spectrum. A new CNN architecture including a reversible down- and up-sampling (DU) operator and a loss function based on proper orthogonal decomposition (POD) coefficients is proposed. For training and testing the CNN, flame chemiluminescence spectra were captured from a stable methane-air flat flame using a portable spectrometer (spectral range: 250 - 850 nm, resolution: 0.5 nm) with varied equivalence ratio (0.8 - 1.2), pressure (1 - 10 bar), and exposure time (0.05, 0.2, 0.4, and 2 s). The long exposure (2 s) spectra were used as the ground truth when training the denoising CNN. A kriging model with POD is trained by the long-gated spectra for calibration, and then the prediction of the gas properties taking the denoised short-gated spectrum as the input: The property prediction errors of pressure and equivalence ratio were remarkably lowered in spite of the low SNR attendant with reduced exposure.